Publication

Nanoparticle discrimination based on wavelength and lifetime-multiplexed cathodoluminescence microscopy

Garming, M. W. H., Weppelman, I. G. C., de Boer, P., Martínez, F. P., Schirhagl, R., Hoogenboom, J. P. & Moerland, R. J. 14-Sep-2017 In : Nanoscale. 9, 34, p. 12727-12734 8 p.

Research output: Scientific - peer-reviewArticle

APA

Garming, M. W. H., Weppelman, I. G. C., de Boer, P., Martínez, F. P., Schirhagl, R., Hoogenboom, J. P., & Moerland, R. J. (2017). Nanoparticle discrimination based on wavelength and lifetime-multiplexed cathodoluminescence microscopy. Nanoscale, 9(34), 12727-12734. DOI: 10.1039/c7nr00927e

Author

Garming, Mathijs W H; Weppelman, I Gerward C; de Boer, Pascal; Martínez, Felipe Perona; Schirhagl, Romana; Hoogenboom, Jacob P; Moerland, Robert J / Nanoparticle discrimination based on wavelength and lifetime-multiplexed cathodoluminescence microscopy.

In: Nanoscale, Vol. 9, No. 34, 14.09.2017, p. 12727-12734.

Research output: Scientific - peer-reviewArticle

Harvard

Garming, MWH, Weppelman, IGC, de Boer, P, Martínez, FP, Schirhagl, R, Hoogenboom, JP & Moerland, RJ 2017, 'Nanoparticle discrimination based on wavelength and lifetime-multiplexed cathodoluminescence microscopy' Nanoscale, vol 9, no. 34, pp. 12727-12734. DOI: 10.1039/c7nr00927e

Standard

Nanoparticle discrimination based on wavelength and lifetime-multiplexed cathodoluminescence microscopy. / Garming, Mathijs W H; Weppelman, I Gerward C; de Boer, Pascal; Martínez, Felipe Perona; Schirhagl, Romana; Hoogenboom, Jacob P; Moerland, Robert J.

In: Nanoscale, Vol. 9, No. 34, 14.09.2017, p. 12727-12734.

Research output: Scientific - peer-reviewArticle

Vancouver

Garming MWH, Weppelman IGC, de Boer P, Martínez FP, Schirhagl R, Hoogenboom JP et al. Nanoparticle discrimination based on wavelength and lifetime-multiplexed cathodoluminescence microscopy. Nanoscale. 2017 Sep 14;9(34):12727-12734. Available from, DOI: 10.1039/c7nr00927e


BibTeX

@article{6598da3ba3184abfa602f4a5ab295f3b,
title = "Nanoparticle discrimination based on wavelength and lifetime-multiplexed cathodoluminescence microscopy",
abstract = "Nanomaterials can be identified in high-resolution electron microscopy images using spectrally-selective cathodoluminescence. Capabilities for multiplex detection can however be limited, e.g., due to spectral overlap or availability of filters. Also, the available photon flux may be limited due to degradation under electron irradiation. Here, we demonstrate single-pass cathodoluminescence-lifetime based discrimination of different nanoparticles, using a pulsed electron beam. We also show that cathodoluminescence lifetime is a robust parameter even when the nanoparticle cathodoluminescence intensity decays over an order of magnitude. We create lifetime maps, where the lifetime of the cathodoluminescence emission is correlated with the emission intensity and secondary-electron images. The consistency of lifetime-based discrimination is verified by also correlating the emission wavelength and the lifetime of nanoparticles. Our results show how cathodoluminescence lifetime provides an additional channel of information in electron microscopy.",
keywords = "SCANNING-ELECTRON-MICROSCOPE, NITROGEN-VACANCY CENTERS, FLUORESCENT NANODIAMONDS, HIGH-RESOLUTION, BEAM EXCITATION, PHOTOLUMINESCENCE, IDENTIFICATION, MOLECULES, DENSITY, DIAMOND",
author = "Garming, {Mathijs W H} and Weppelman, {I Gerward C} and {de Boer}, Pascal and Martínez, {Felipe Perona} and Romana Schirhagl and Hoogenboom, {Jacob P} and Moerland, {Robert J}",
year = "2017",
month = "9",
doi = "10.1039/c7nr00927e",
volume = "9",
pages = "12727--12734",
journal = "Nanoscale",
issn = "2040-3364",
publisher = "ROYAL SOC CHEMISTRY",
number = "34",

}

RIS

TY - JOUR

T1 - Nanoparticle discrimination based on wavelength and lifetime-multiplexed cathodoluminescence microscopy

AU - Garming,Mathijs W H

AU - Weppelman,I Gerward C

AU - de Boer,Pascal

AU - Martínez,Felipe Perona

AU - Schirhagl,Romana

AU - Hoogenboom,Jacob P

AU - Moerland,Robert J

PY - 2017/9/14

Y1 - 2017/9/14

N2 - Nanomaterials can be identified in high-resolution electron microscopy images using spectrally-selective cathodoluminescence. Capabilities for multiplex detection can however be limited, e.g., due to spectral overlap or availability of filters. Also, the available photon flux may be limited due to degradation under electron irradiation. Here, we demonstrate single-pass cathodoluminescence-lifetime based discrimination of different nanoparticles, using a pulsed electron beam. We also show that cathodoluminescence lifetime is a robust parameter even when the nanoparticle cathodoluminescence intensity decays over an order of magnitude. We create lifetime maps, where the lifetime of the cathodoluminescence emission is correlated with the emission intensity and secondary-electron images. The consistency of lifetime-based discrimination is verified by also correlating the emission wavelength and the lifetime of nanoparticles. Our results show how cathodoluminescence lifetime provides an additional channel of information in electron microscopy.

AB - Nanomaterials can be identified in high-resolution electron microscopy images using spectrally-selective cathodoluminescence. Capabilities for multiplex detection can however be limited, e.g., due to spectral overlap or availability of filters. Also, the available photon flux may be limited due to degradation under electron irradiation. Here, we demonstrate single-pass cathodoluminescence-lifetime based discrimination of different nanoparticles, using a pulsed electron beam. We also show that cathodoluminescence lifetime is a robust parameter even when the nanoparticle cathodoluminescence intensity decays over an order of magnitude. We create lifetime maps, where the lifetime of the cathodoluminescence emission is correlated with the emission intensity and secondary-electron images. The consistency of lifetime-based discrimination is verified by also correlating the emission wavelength and the lifetime of nanoparticles. Our results show how cathodoluminescence lifetime provides an additional channel of information in electron microscopy.

KW - SCANNING-ELECTRON-MICROSCOPE

KW - NITROGEN-VACANCY CENTERS

KW - FLUORESCENT NANODIAMONDS

KW - HIGH-RESOLUTION

KW - BEAM EXCITATION

KW - PHOTOLUMINESCENCE

KW - IDENTIFICATION

KW - MOLECULES

KW - DENSITY

KW - DIAMOND

U2 - 10.1039/c7nr00927e

DO - 10.1039/c7nr00927e

M3 - Article

VL - 9

SP - 12727

EP - 12734

JO - Nanoscale

T2 - Nanoscale

JF - Nanoscale

SN - 2040-3364

IS - 34

ER -

ID: 47023246